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Anne L'Huillier

Anne l'Huillier

Professor

Anne L'Huillier

Calculations of high-order harmonic-generation processes in xenon at 1064 nm

Author

  • Anne LHuillier
  • Philippe Balcou
  • Sebastien Candel
  • Kenneth J. Schafer
  • Kenneth C. Kulander

Summary, in English

We perform detailed calculations of harmonic conversion in a 15-Torr jet of xenon into which a 1064-nm-wavelength 36-ps-pulse-width laser has been tightly focused, so that the peak intensity ranges from 5×1012 to 5×1013 W cm-2. The single-atom emission rates are obtained by integrating the time-dependent Schrödinger equation. We employ an improved atomic model which includes excitation and ionization through states with both low-lying ionic cores. The propagation equations are solved using a general and efficient finite-difference technique. Excellent agreement with experimental data is obtained. We consider the effect of the defocusing of the pump beam by the free electrons in the saturation regime, and find it to be small for the conditions studied here. The spatial, temporal, and spectral profiles of the harmonic emission are presented. Significant blueshifts of the harmonics spectral line shapes are observed in the saturation regime. Finally, using model polarizations, we discuss how the harmonic fields build up in the nonlinear medium, through a series of interferences. It allows us to understand why efficient phase matching can be achieved in a strong-field regime for the laser-atom interaction.

Publishing year

1992-09

Language

English

Pages

2778-2790

Publication/Series

Physical Review A

Volume

46

Issue

5

Document type

Journal article

Publisher

American Physical Society

Topic

  • Atom and Molecular Physics and Optics

Status

Published

ISBN/ISSN/Other

  • ISSN: 1050-2947